The problem is solved!
In short, only Visual Studio 2010 Service Pack 1 is missing, and the DLL does not contain a method that is called using the test controller configuration tool.
Solution: Install Windows 2010 Service Pack 1 (SP1).
Reason: Microsoft.VisualStudio.QualityTools.LoadTest.DLL does not contain a database validation method that is called by the configuration tool, so an exception is thrown and the configuration does not work. After upgrading to SP1, the DLL is updated successfully, and the missing method can be found there.
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